Prompt Gamma Activation Analysis of $^{188}$RE

ORAL

Abstract

Prompt $\gamma$ activation analysis was used to determine partial $\gamma$ production cross sections from the $^{187}$Re(n,$\gamma$)$^{188}$Re reaction at the Budapest Neutron Centre in Budapest, Hungary. The 10-MW$_{t}$ research reactor provided the source of neutrons, which were cooled to a spectrum of $\sim$140 K and collimated onto a target of powdered rhenium metal enriched to 99.52\% $^{187}$Re. Prompt $\gamma$ spectra were collected with a single Compton-suppressed HPGe detector. Subsequent fitting of the raw spectral data produced precise energies and intensities of the observed transitions. The $^{188}$Re cross sections were determined by standardizing measured peak intensities to well-known $^{35}$Cl(n,$\gamma$)$^{36}$Cl cross sections via a second spectrum from a sample of ReCl$_{3}$. However, the non-trivial volume of the enriched sample resulted in energy-dependent self-attenuation of $\gamma$-rays originating in the sample bulk. This necessitated estimating the effective optical thickness of the enriched sample to derive intensity adjustments, particularly for $\gamma$-rays below $\sim$300 keV. Forthcoming analysis will use statistical decay modeling to predict the population of known levels from the neutron-capture state for comparison with observed cross sections.

Authors

  • T. W. Warren

    • Air Force Institute of Tech - WPAFB
  • D. A. Matters

    • Defense Threat Reduction Agency
  • A. M. Hurst

    • Lawrence Berkeley Laboratory
  • L. Szentmiklosi

    • Budapest Neutron Centre
  • J. J. Carroll

    • U. S. Army Research Laboratory
  • J. W. McClory

    • Air Force Institute of Tech - WPAFB
  • T. Belgya

    • Budapest Neutron Centre