\textit{Ab initio} exploration of the frequency comb structure and coherence in high-order harmonics of multi-electron systems driven by a sequence of ultrashort laser pulses
POSTER
Abstract
We present an \textit{ab initio }nonpertubative investigation of the frequency comb structure and coherence within each order of the high harmonic generation (HHG) of rare gas atoms by means of the self-interaction-free time dependent density functional theory (TDDFT). The time-dependent exchange-correlation potential is constructed by means of the time dependent optimized effective potential (TDOEP) method. The TDOEP equations are solved accurately and efficiently by means of the time-dependent generalized pseudospectral technique. We explore in detail the temporal coherence and robustness of the comb structure by varying the laser pulse duration $t$, the number of pulses $N$, and the laser intensity. We found that a nested comb structure appears within each order of the harmonics, ranging from the first harmonic all the way to the cut-off harmonic, and this global pattern persists regardless of the values of $t$ and $N$ used, and even in the presence of substantial ionization.
Authors
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Juan J. Carrera
Center for Theoretical Sciences, Dept. of Physics, National Taiwan University, Taipei, Taiwan
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Shih-I Chu
Center for Theoretical Sciences, Dept. of Physics, National Taiwan University, Taipei, Taiwan, University of Kansas, Dept. of Chemistry, Univ. of Kansas, Lawrence, KS 66045 USA, Department of Chemistry, University of Kansas, Department of Chemistry, University of Kansas, Lawrence, KS 66045