100-fold improvement on Atom Trap Trace Analysis for radiokrypton dating
POSTER
Abstract
Atom Trap Trace Analysis (ATTA) has been used to analyze the rare isotope Kr-81 (half-life = 230 kyrs, I.A.$\sim $ 10$^{-13})$ in environmental samples. Kr-81 analysis can now be used to determine the ages of groundwater samples in the range of 50 -- 1,000 kyrs. The previous instrument (ATTA-2) had an overall counting efficiency of 0.01{\%} and, required a water sample of 1,000 liters. We are developing a new instrument (ATTA-3) to laser-trap and count Kr-81 atoms with the goal of reaching a counting efficiency of 1{\%}, which would reduce the sample size to less than 100 liters of water or ice. Recently we have demonstrated a counting rate of $\sim $ 2000 $^{81}$Kr atoms/hr, which represents a 100-fold improvement over ATTA-2. ATTA-3 will enable a wide range of applications in the earth sciences.
Authors
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W. Jiang
Argonne National Lab (ANL)
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W. Williams
Physics Div, Argonne National Lab, ANL
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Y.R. Sun
HFNL, Univ of Sci \& Tech of China (USTC)
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K. Bailey
ANL
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A.M. Davis
EFI, Univ of Chicago; Univ of Chicago (U of C)
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S.-M. Hu
HFNL, USTC
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Z.-T. Lu
Physics Div, Argonne National Lab and Dept of Physics, Univ of Chicago, Argonne National Laboratory, ANL; EFI, Univ of Chicago; U of C
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P. Mueller
Physics Div, Argonne National Lab, ANL
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T.P. O'Connor
ANL
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R. Purtschert
Univ of Bern
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N.C. Sturchio
Univ of Illinois at Chicago