Dissociative ionizaiton of $H_2$ in an ultroviolet pulse train and delayed infrared laser pulse
ORAL
Abstract
The ionization of H$_2$ in a single attosecond XUV pulse generates a nuclear wavepacket in H$_2^+$ which is entangled with the emitted photoelectron wavepacket. The nuclear wavepacket dynamics can be observed by dissociating H$_2^+$ in a delayed infrared laser pulse. If H$_2$ is ionized by a sequence of XUV pulses of an attosecond pulse train, whether or not the corresponding sequence of nuclear wavepackets in H$_2^+$ is detected as a coherent or incoherent superposition depends on whether and how the photoelectrons are observed. We simulate the nuclear dynamics in this XUV pump - IR probe scenario and analyze our numerical results, suggesting that interference between coherently launched nuclear wavepackets in H$_2^+$ can be neglected in the recent experiment of Kelkensberg \textit{et al.} [\textbf{103}, 123005 (2009)].
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Authors
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Feng He
James R. Macdonald Laboratory, Kansas State University
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Uwe Thumm
James R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506-2604, USA, James R. Macdonald Laboratory, Kansas State University, Kansas State University, Manhattan, KS 66502, Kansas State University