Centrifugal Distortion Causes Anderson Localization in Laser Kicked Molecules

ORAL

Abstract

The periodically kicked 2D rotor is a textbook model in nonlinear dynamics. The classical kicked rotor can exhibit truly chaotic motion, whilst in the quantum regime this chaotic motion is suppressed by a mechanism similar to Anderson Localization. Up to now, these effects have been mainly observed in an atom optics analogue of a quantum rotor: cold atoms in a standing light wave. We demonstrate that common linear molecules (like N$_2$, O$_2$, CO$_2$, ...), kicked by a train of short linearly polarized laser pulses, can exhibit a new mechanism for dynamical Anderson Localization due to their non-rigidity. When the pulses are separated by the rotational revival time $t_{rev}=\pi\hbar/B$, the angular momentum $J$ grows ballistically (Quantum Resonance). We show that, due to the centrifugal distortion of fast spinning molecules, above some critical value $J=J_{cr}$ the Quantum Resonance is suppressed via the mechanism of Anderson Localization. This leads to a non-sinusoidal oscillation of the angular momentum distribution, which may be experimentally observed even at ambient conditions by using current techniques for laser molecular alignment.

Authors

  • Johannes Floss

    Weizmann Institute of Science

  • Ilya Sh. Averbukh

    Weizmann Institute of Science