Spin Dynamics of Two-Dimensional&nbsp;V<sub>B</sub><sup>-&nbsp;</sup>Ensembles in Hexagonal Boron Nitride

POSTER

Abstract

Strongly interacting color-center ensembles are conventionally realized in three-dimensional systems. While these systems have been widely used as quantum sensors and as simulator platforms for studying many-body dynamics, accessing lower-dimensional physics with solid-state color centers remains an open challenge. Here, we investigate the many-body dynamics of ensembles of negatively charged boron vacancy (VB-) defects in few-layer hexagonal boron nitride (hBN) flakes, where the flake thickness is smaller than the average inter-defect spacing. In this regime, we show that the emergent dynamics are governed by native dipolar interactions between the VBdefects. In particular, we employ a form of many-body noise spectroscopy in which the system dimensionality directly manifests in the temporal profile of VBdecoherence dynamics. Building on this, we measure local spin–spin autocorrelation functions to probe and compare spin transport in two-dimensional thin flakes and three-dimensional bulk ensembles.

Presenters

  • Wonjae Lee

    • Harvard University

Authors

  • Wonjae Lee

    • Harvard University
  • Zhelun Zhang

    • Harvard University
  • Sangha Kim

    • Harvard University
  • Jonathan N Hallén

    • Harvard University
  • Vincent Liu

    • Harvard University
  • Ruotian Gong

    • Washington University in St. Louis
  • Thomas Poirier

    • Kansas State University
  • James Edgar

    • Kansas State University
  • Chong Zu

    • Washington University, St. Louis
  • Norman Y Yao

    • Harvard University