Cold Chemistry and Optical Cycling in CH Radicals

ORAL

Abstract

Recent advances in molecular laser cooling have opened new opportunities for quantum control across a wide range of species. We extend these techniques to CH, a light organic radical whose electronic structure offers diagonal Franck-Condon factors on the X-A transition. The low mass and blue-wavelength cycling transition in CH enables a large photon recoil velocity, reducing the required photon budget and rovibrational closure needed to load a magneto‑optical trapping. Our experiment aims to leverage these features to develop a platform for studies of ultracold organic chemistry. We will present an experimental update, including measurements of cold organic chemistry in our cryogenic source and results demonstrating optical cycling.

**This work is supported by the AFOSR (FA9550-22-1-0277) and a DURIP award (FA9550-23-1-0074).

Presenters

  • Aritra Paul

    • University of Connecticut

Authors

  • Aritra Paul

    • University of Connecticut
  • Alexander T Preston

    • University of Connecticut
  • Daniel McCarron

    • University of Connecticut