<sup>236</sup>U/<sup>238</sup>U Isotopic Ratio Measurements with Accelerator Mass Spectrometry Using the USRM Standard Reference Materials
ORAL
Abstract
236U is a rare isotope of uranium, naturally occurring in ores with an isotopic abundance of 236U/natU<1x10-9 and anthropogenically occurring in soil and water systems as high as 236U/238U = 1x10-3. Its natural abundance varies over a few orders of magnitude between different mine locations and any individual location’s abundance of 236U has long been considered a unique “fingerprint”-like signature. Only Accelerator Mass Spectrometry (AMS) is capable of measuring this abundance across the full range of natural 236U abundances. In order to make these measurements more repeatable, and increase accuracy across different AMS facilities, the AMS group at the University of Notre Dame has prepared a series of 236U reference standards that covers the isotope’s natural abundance range. Verification measurements of standard series will be presented alongside measurements of ores across the continental United States and the Vienna-KkU reference standard. Additionally a detection limit of 1x10-12 was determined.
*This work is supported by the National Science Foundation Grant No. NSF PHY-2011890, the Nuclear Regulatory Commission Award No. 31310019M0037, and the National Nuclear Security Administration, Grant No. NA0004093. I.A. Russell was supported by the Consortium for Nuclear Forensics, which receives funding from the National Nuclear Security Administration under grant number DE-NA0004142.
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Publication: Producing 236U reference standards for Accelerator Mass Spectrometry at the University of Notre Dame
Presenters
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Thomas L Bailey
- University of Notre Dame