Ultra-fast Measurements of Optically Induced Lattice Dynamics in LuMnO$_3$ Using Aluminum K-alpha X-Ray Diffraction.

POSTER

Abstract

An experiment to study the structural dynamics at the ultra-fast time scale in optically-pumped samples is presented. Measurements of lattice dynamics in LuMnO$_3$ are presented and compared to calculations using dynamical diffraction theory modified for hexagonal crystal structure. Ultra-fast x-ray emission is used to measure Bragg peak shifts using diffraction and compared to calculations. Results are presented for optical pump energy densities of 8 and 20-mJ/cm$^{2}$. The experiment uses $\sim $150 mJ of a 100fs Ti:Sapphire laser to excite K-alpha x-ray emission in an aluminum wire with $\sim $1-2{\%} split off for the material pump. The x-ray emission is relayed using a spherical Quartz crystal to the sample target. Plans for experiments using Cu K-alpha emission to probe Fe samples will also be described.

*Work performed under the auspices of the Dept. of Energy under contract \# W-7405-ENG-36.

Authors

  • J. Workman

  • H.J. Lee

  • J. Roberts

  • Q. McCulloch

  • A.J. Taylor

  • D.J. Funk

    • Los Alamos National Laboratory
  • J.S. Wark

    • Clarendon Laboratory, University of Oxford