Measuring Dynamic Properties of Warm Dense Matter with High-Resolution Inelastic X-ray Scattering

ORAL

Abstract

Warm dense matter (WDM) is a complex state of matter where strong ion-ion coupling combined with the quantum behavior of the electron fluid make simulation and modeling challenging; experimental verification in this regime is essential. X-ray scattering experiments, which utilize high-intensity beams of penetrating radiation to probe the micro-structure and dynamics, allow for critical testing of our simulations. I will provide an overview of our high-resolution (∼50 meV) X-ray scattering platform, designed for use with free-electron lasers, with a resolution capable of measuring the quasi-elastic Rayleigh peak (in the non-collective regime) and discerning ion modes (in the collective regime). In the first case, we have directly measured the electron-ion equilibration rate in various laser-excited metallic thin films (Au, Ag, Cu, and Ti). In the latter, we have successfully measured the sound speed in warm dense methane.

*This work was funded in part by the U.S. Department of Energy, NNSA under Award No. DE-NA0004039. Use of the LCLS is supported by the U.S. DOE, Office of Science, Office of BES under Contract No. DE-AC02-76SF00515. The MEC instrument is supported by the U.S. Department of Energy, Office of Science, Office of FES under contract No. DE-AC02-76SF00515.

Publication: T. G. White et al. Observation of Ion Acoustic Waves in Warm Dense Methane. To be submitted to PRL before APS-DPP.
D. Haden et al. Electron-Ion Equilibration in Warm Dense Gold, Silver, and Nickel. In Prep.
A. Descamps et al. J. Synchrotron Rad. (2022). 29, 931-938
L. Wollenwebber et al. Review of Scientific Instruments 92, 013101 (2021)
E.E. McBride et al. Review of Scientific Instruments 89, 10F104 (2018)

Presenters

  • Thomas G White

    • University of Nevada, Reno

Authors

  • Thomas G White

    • University of Nevada, Reno
  • Daniel Haden

    • University of Nevada, Reno
  • Emma E McBride

    • SLAC
    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Karen Appel

    • European XFEL GmbH
  • Ben Armentrout

    • SLAC National Accelerator Laboratory
  • Florian Condamine

    • ELI Beamlines
    • ELI-Beamlines Center, Institute of Physics, Czech Academy of Sciences, 25241 Dolní Brežany, Czech Republic
    • ELI Beamlines, Prague, Czech Republic
  • Carson Convery

    • SLAC National Accelerator Laboratory
  • Eric Cunningham

    • SLAC National Accelerator Laboratory
    • SLAC - Natl Accelerator Lab
  • Chandra Breanne Curry

    • SLAC National Accelerator Laboratory
  • Francesco Dallari

    • University of Trento
  • Adrien Descamps

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Luke Fletcher

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Stefan Funk

    • Friedrich-Alexander University Erlangen-Nürnberg
  • Eric Galtier

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Maxence Gauthier

    • SLAC National Accelerator Laboratory
    • SLAC - Natl Accelerator Lab
  • Dirk Gericke

    • University of Warwick
  • Sebastian Goede

    • European XFEL GmbH
    • European XFEL
  • Jerome B Hastings

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Dimitri Khaghani

    • SLAC National Accelerator Laboratory
    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Accelerator
  • Jongjin B Kim

    • SLAC National Accelerator Laboratory
  • Haeja Lee

    • SLAC National Accelerator Laboratory
    • SLAC - Natl Accelerator Lab
  • Jacob M Molina

    • University of Nevada, Reno
  • Giulio Monaco

    • University of Trento
  • Benjamin K Ofori-Okai

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Hannah Poole

    • University of Oxford
  • Christopher Schoenwaelder

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Peihao Sun

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Thomas Tschentscher

    • European XFEL
  • Bastian Witte

    • University of Rostock
  • Sameen Yunus

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Lennart Wollenweber

    • European XFEL GmbH
    • European XFEL
  • Ulf Zastrau

    • European XFEL GmbH
    • European XFEL
  • Siegfried H Glenzer

    • SLAC National Accelerator Laboratory
    • SLAC - Natl Accelerator Lab
    • Lawrence Livermore Natl Lab
  • Bob Nagler

    • SLAC - Natl Accelerator Lab
    • SLAC National Accelerator Laboratory
  • Gianluca Gregori

    • University of Oxford