Probing ionization in warm dense copper using x-ray absorption spectroscopy

ORAL

Abstract

Warm dense matter exists at temperatures of order 10 eV and a few times solid density, where the complex balance of collective and quantum effects precludes standard approximations used in plasma physics or condensed matter physics. Understanding ionization in the warm dense matter regime, in particular, is an active area of research requiring additional experimental data to benchmark and improve current predictive capabilities. In this study, we present the experimental results and analysis of K-shell x-ray absorption spectra to infer temperature and ionization state distribution of copper uniformly heated to temperatures 10–30 eV and compressed to densities of 9–30 g/cm3. The experiments were conducted at the OMEGA laser facility using a buried layer of copper tamped by plastic on both sides, where the two sides were then irradiated by a symmetric laser drive and probed by a broadband x-ray source. Experimental results are compared to collisional-radiative models where we find large discrepancies in the predicted x-ray absorption spectra at these conditions. We also explore the role of including density effects in the underlying atomic data used in the collisional-radiative models and compare the results to our experimental data.

*This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and was supported by the LLNL-LDRD Program under Project No. 22-ERD-005. SNL is managed and operated by NTESS under DOE NNSA contract DE-NA0003525. LLNL-ABS-866224.

Presenters

  • Tanner Cordova

    • University of California San Diego

Authors

  • Tanner Cordova

    • University of California San Diego
  • Mike J MacDonald

    • Lawrence Livermore Natl Lab
    • Lawrence Livermore National Laboratory
  • Edward V Marley

    • Lawrence Livermore National Laboratory
  • D. A. Alexander Chin

    • University of Rochester
    • Laboratory for Laser Energetics
  • Tilo Doeppner

    • LLNL
    • Lawrence Livermore National Laboratory
  • Richard A London

    • Lawrence Livermore Natl Lab
  • Michael K Kruse

    • Lawrence Livermore National Laboratory
    • Lawrence Livermore Natl Lab
  • Howard A Scott

    • Lawrence Livermore National Laboratory
  • Farhat N Beg

    • University of California, San Diego
    • UC San Diego
  • Federica Coppari

    • Lawrence Livermore Natl Lab
  • Jim A Emig

    • Lawrence Livermore Natl Lab
  • Stephanie B Hansen

    • Sandia National Laboratories
  • Marius Millot

    • LLNL
    • Lawrence Livermore National Laboratory
  • Philip M Nilson

    • Lab for Laser Energetics
  • Philip A Sterne

    • Lawrence Livermore National Laboratory
    • Lawrence Livermore Natl Lab