Measure of temperature and ionization in warm dense mid-Z metal alloys using x-ray absorption spectroscopy

POSTER

Abstract

Warm dense matter exists at temperatures of order 10 eV and a few times solid density, where the complex balance of collective and quantum effects precludes standard approximations used in plasma physics or condensed matter physics. Understanding ionization in the warm dense matter regime, in particular\, is an active area of research that requires additional experimental data to benchmark and improve current predictive capabilities. In this study, we present the experimental results and analysis of K-shell x-ray absorption spectra. X-ray absorption is used to extract an inference of the charge state distribution and electron temperature. Targets comprised of copper, brass, and copper-aluminum were uniformly heated to temperatures 10–40 eV and compressed to densities of 5–25 g/cm3. The variation in the fraction of copper allows for exploration of density variations on ionization. The experiments were conducted at the OMEGA laser facility using a buried layer of copper, or copper alloy, tamped by plastic on both sides. The two sides were then irradiated by symmetric laser pulses and probed by a laser-generated x-ray source. Experimental results are compared to collisional-radiative models, where we find large discrepancies in the predicted x-ray absorption spectra at these conditions. We also explore the role of including density effects in the underlying atomic data used in the collisional-radiative models and compare the results to our experimental data.

*This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and was supported by the LLNL-LDRD Program under Project No. 22-ERD-005. SNL is managed and operated by NTESS under DOE NNSA contract DE-NA0003525. LLNL-ABS-868920

Presenters

  • Tanner Cordova

    • University of California San Diego

Authors

  • Tanner Cordova

    • University of California San Diego
  • Mike J MacDonald

    • Lawrence Livermore National Laboratory
  • Ed V Marley

    • Lawrence Livermore National Laboratory
  • David Alexander Chin

    • University of Rochester
    • Laboratory for Laser Energetics
    • Laboratory for Laser Energetics, University of Rochester, Rochester, NY, United States
  • Tilo Doeppner

    • Lawrence Livermore National Laboratory
  • Richard A London

    • Lawrence Livermore National Laboratory
  • Veronika K Kruse

    • Lawrence Livermore National Laboratory
  • Howard A Scott

    • Lawrence Livermore National Laboratory
  • Farhat N Beg

    • University of California, San Diego
  • Federica Coppari

    • Lawrence Livermore National Laboratory
  • Jim A Emig

    • Lawrence Livermore Natl Lab
  • Stephanie B Hansen

    • Sandia National Laboratories
  • Carolyn C Kuranz

    • University of Michigan
    • OCC
  • Marius Millot

    • Lawrence Livermore National Laboratory
  • Philip M Nilson

    • Laboratory for Laser Energetics (LLE)
  • Michael Springstead

    • University of Michigan
  • Philip A Sterne

    • Lawrence Livermore National Laboratory