Replica theory for fluctuations of the activation barriers in glassy systems

ORAL

Abstract

Using an effective potential approach to self generated glasses we determine the nucleation of entropic droplets in systems with random first order transition and entropy crisis. We demonstrate that fluctuations of the configurational entropy and of the liquid glass surface tension are crucial for an understanding of the barrier fluctuations in glassy systems and thus are responsible for the broad spectrum of excitations and heterogeneous dynamics in glasses. In particular we derive a relation between the length scale for dynamic heterogeneity and the related barrier fluctuations.

Authors

  • Joerg Schmalian

    Iowa State University, Ames Laboratory and Department of Physics \& Astronomy, Iowa State University, Ames IA 50011, Ames Lab and Iowa State University

  • Maxim Dzero

    Rutgers University

  • Peter Wolynes

    University of California at San Diego