Griffiths phase and parimagnetism in ErCo$_{2}$
ORAL
Abstract
A systematic study of the paramagnetic phase of ErCo$_{2}$ has recently allowed to identify the inversion of the net magnetization of the Co net moment with respect to the applied field well above the ferrimagnetic ordering temperature, $T_{C}$. This phenomenon, which we have denoted \textit{parimagnetism}, may be related with the onset of a Griffiths-like phase in paramagnetic ErCo$_{2}$. We have measured SANS and ac susceptibility on ErCo$_{2}$ as a function of temperature, applied field, and excitation frequency. Several characteristics shared by systems showing a Griffiths phase are present in ErCo$_{2}$, namely the formation of ferromagnetic clusters in the disordered phase, the loss of analyticity of the magnetic susceptibility and its extreme sensitivity to an applied field. Our XMCD study of the Co magnetic moment flipping process show the ocurrence of a pseudo-violation of the third Hund's rule at the para- to parimagnetic ``transition''.
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Authors
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Fernando Bartolome
ICMA, CSIC - Universidad de Zaragoza
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Luis M. Garcia
ICMA, CSIC - Universidad de Zaragoza
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Julia Herrero-Albillos
Materials Science Dept., Cambridge University
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Anthony T. Young
Advanced Light Source, LBNL
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Tobias Funk
UCSF Physics Research Laboratory