Magnetic and Structural Properties of Sr-Doped Ba$_{2-x}$Sr$_{x}$CoO$_{4}$

ORAL

Abstract

We have studied the structural and magnetic properties of a newly synthesized compound Ba$_{2-x}$Sr$_{x}$CoO$_{4}$ with different doping ($x)$ levels. Monoclinic Ba$_{2}$CoO$_{4}$ is an antiferromagnetic (AFM) insulator with N\'eel temperature $T_{N}$ = 25 K and a two-dimensional character with spins aligned in the \textit{ac} plane. The isovalent Sr doping causes changes in both crystal structure and magnetic properties. With increasing $x$, $T_{N}$ initially increases then decreases after reaching the maximum at $x$=0.5. Correspondingly, its crystal structure changes from monoclinic ($x <$ 0.5) to orthorhombic ($x\ge $0.5) at room temperature. The correlation between crystal structure and physical properties will be discussed.

Authors

  • Hao Sha

    Department of Physics, Florida International University, Miami, FL 33199, Florida International University, Miami, FL 33199

  • Jiandi Zhang

    Department of Physics, Florida International University, Miami, FL 33199, Florida International University, Miami, FL 33199, Florida International University, Florida International University (FIU), Miami, FL 33199

  • Qingzhen Huang

    NIST Center for Neutron Research, NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, National Institute of Standards and Technology (NCNR)

  • Ovidiu Garlea

    Neutron Scattering Science Division, ORNL, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge national laboratory, Oak Ridge National Laboratory

  • B.C. Sales

    Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge TN 37831

  • David Mandrus

    Materials Science and Technology Division, ORNL, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge TN 37831, Oak Ridge Natl Lab

  • Ronying Jin

    Materials Science and Technology Division, ORNL, Oak Ridge, TN 37831 and Univ. of Tennessee, Knoxville, TN 37996, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge TN 37831, Oak Ridge National Laboratory