Anomalous nuclear relaxation in the ferromagnetic phase of the bilayered manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$.

ORAL

Abstract

In contrast to ferromagnetic (FM) 3D manganites, $^{55}$Mn NMR spectra obtained for the FM phase of the colossal magnetoresistance bilayer manganite La$_{1.2 }$Sr$_{1.8 }$Mn$_{2}$O$_{7}$ show a broad distribution of hyperfine fields implying a large distribution of local environments at Mn sites. The hyperfine distribution may be linked to orbital ordering effects. $^{55}$Mn spin -- lattice relaxation rates have a surprisingly weak dependence both on temperature and applied magnetic field. Significant departures of the relaxation rate from Korringa temperature dependence below 20 K provide evidence for non-Fermi liquid behavior in this quasi-2D metal. At temperatures approaching $T_{C }$ from below, further anomalous behavior is found consistent with spin polaron formation in the range where colossal magnetoresistance starts to appear.

Authors

  • Michael Hoch

    National High Magnetic Field Laboratory, 1800 E. Paul Dirac Dr., Tallahassee, FL 32310

  • Philip Kuhns

    National High Magnetic Field Laboratory, Tallahassee, FL, USA, NHMFL/FSU, National High Magnetic Field Laboratory, 1800 E. Paul Dirac Dr., Tallahassee, FL 32310

  • William Moulton

    National High Magnetic Field Laboratory, 1800 E. Paul Dirac Dr., Tallahassee, FL 32310

  • Arneil Reyes

    National High Magnetic Field Laboratory, Tallahassee, FL, USA, National High Magnetic Field Lab, NHMFL/FSU, National High Magnetic Field Laboratory, 1800 E. Paul Dirac Dr., Tallahassee, FL 32310

  • Jun Lu

    National High Magnetic Field Laboratory, 1800 E. Paul Dirac Dr., Tallahassee, FL 32310

  • John Mitchell

    Argonne National Laboratory, Materials Science Division, Argonne National Laboratory, Argonne National Laboratory, Argonne, IL 60439