Apparent anomaly in electron scattering in Ag nanostructures*

ORAL

Abstract

Electron scattering from diffusing atoms can be visualized via the effects of the corresponding force that biases atomic motion, the ``electromigration force''. Using a combination of scanning tunneling microscopy and scanning electron microscopy, we investigate electron scattering via the biased motion of monatomic islands and C$_{60}$-decorated steps on Ag(111) surfaces in the presence of large current density (j$_{bulk}$ = 6.7x10$^{9}$ A/m$^{2})$. For monatomic adatom islands, the biased motion is opposite to the current direction and thus parallel to the direction of momentum transfer (the ``wind force'' direction), while vacancy islands move oppositely. The measured drift velocity v as a function of the island radius R, vR = 1.9nm$^{2}$/s, yields an anomalously large$^{1}$ effective force per boundary atom $\sim $0.06 meV/nm . An effective scattering force of similar magnitude is also observed via current-induced curvature of C$_{60}$ decorated line-boundaries. Possible mechanisms for this effect, including current crowding, charge transfer and local heating, will be discussed. 1. A. Bondarchuk, et al. Phys. Rev. Lett. \textbf{99, 206801 (2007)}

Authors

  • Ellen Williams

    University of Maryland, College Park, Department of Physics and University of Maryland Materials Research Science and Engineering Center, University of Maryland, College Park, MD 20742, University of Maryland, LPS, CNAM, and the DOP, UM, Physics Department, University of Maryland, College Park, MD 20742, Materials Research Science and Engineering Center, Center for Nanophysics and Advanced Materials, Dept of Physics, Univ. of Maryland, College Park, MD, University of Maryland College Park, Dept. of Physics, U. of Maryland - College Park, Department of Physics and Center for Nanophysics and Advanced Materials, University of Maryland, College Park, MD 20742-4111, USA

  • Chenggang Tao

    Dept. of Physics, U. of Maryland - College Park

  • William G. Cullen

    University of Maryland, Physics Department, University of Maryland, College Park, MD 20742, Materials Research Science and Engineering Center, Center for Nanophysics and Advanced Materials, Dept of Physics, Univ. of Maryland, College Park, MD, University of Maryland College Park, Dept. of Physics, U. of Maryland - College Park