A phase-separation perspective on dynamic heterogeneities in glass-forming liquids

POSTER

Abstract

We study dynamic heterogeneities in a model glass-former whose overlap with a reference configuration is constrained to a fixed value. The system phase-separates into regions of small and large overlap, so that dynamical correlations remain strong even for asymptotic times. We calculate an appropriate thermodynamic potential and find evidence of a Maxwell's construction consistent with a spinodal decomposition of two phases. Our results suggest that dynamic heterogeneities are the expression of an ephemeral phase-separating regime ruled by a finite surface tension.

Authors

  • Chiara Cammarota

    IPhT CEA Saclay France

  • Andrea Cavagna

    SMC ISC CNR-INFM Roma

  • Irene Giardina

    SMC ISC CNR-INFM Roma

  • Giacomo Gradenigo

    SMC CNR-INFM, and Sapienza University Rome

  • Tomas Grigera

    INIFTA, and Universidad Nacional de La Plata, and CCT, La Plata

  • Giorgio Parisi

    SMC CNR-INFM, and Sapienza University Rome

  • Paolo Verrocchio

    Universita di Trento, Trento, and INFM CNR-SOFT, Roma