Nonequilibrium ``melting'' of a charge density wave insulator via an ultrafast infrared laser pulse

ORAL

Abstract

In equilibrium, electrons interacting with lattice vibrations have a transition either to a charge density wave phase (a static modulation of the electronic charge) or to a superconductor (electron pairs move without resistance). If the coupling is weak, the system orders in the Bardeen-Cooper-Schrieffer scenario, where the ordering occurs at some transition temperature Tc and a gap simultaneously forms in the density of states. In strong-coupling, preformed pairs bind at a high temperature (forming a gap in the density of states) and the ordering only occurs at a lower temperature. We employ an exact solution of a model for pump-probe time-resolved photoemission spectroscopy to show how, in nonequilibrium, a third scenario arises: the gap disappears in the presence of a nonzero order parameter, and then reforms well after the pulse has passed. This nonequilibrium ``phase transition'' scenario qualitatively describes all of the available experiments on the ultrafast melting of a charge density wave.

Authors

  • Wen Shen

    Georgetown University

  • Yizhi Ge

    Georgetown University

  • Amy Liu

    Georgetown University, Physics Department, Georgetown University

  • H.R. Krishnamurthy

    Center for Condensed Matter Theory, Indian Institute of Science, Bangalore 560012, India, Department of Physics, Indian Institute of Science, Bangalore 560012, India, India Institute of Science

  • Tom Devereaux

    Department of Physics, Stanford University, Stanford, SIMES, SLAC National Accelerator Laboratory and Stanford University, Stanford Institute for Materials and Energy Science, Stanford Institute for Materials and Energy Science, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA, Stanford Institute for Materials and Energy Science, SLAC National Accelerator Laboratory, Stanford University and SLAC National Accelerator Laboratory, Stanford University

  • Jim Freericks

    Georgetown University