Composition spread studies of (RE)NiO$_{3}$-LaNiO$_{3}$ thin films

ORAL

Abstract

Epitaxial thin films of La$_{x}$Nd$_{1-x}$NiO$_{3}$ and La$_{x}$Pr$_{1-x}$NiO$_{3}$ were grown via pulsed laser deposition on SrTiO$_{3}$ (001) with an automated~moving shutter system to create 100 nm thick composition spreads. These films have the advantage of providing a continuous spectrum of doping compositions at the same deposition conditions, such as temperature and oxygen pressure, without the need to prepare different stoichiometric targets or perform different depositions for desired compositions.~Composition evolution is verified via wavelength dispersive spectroscopy, and x-ray diffraction mapping shows that the lattice constant of the film varies continuously from LaNiO$_{3}$ to NdNiO$_{3}$. Simultaneous measurements of resistance versus temperature down to 4.2 K across the spreads show evolution in transport behavior. The details will be discussed.

Authors

  • Richard Suchoski

    University of Maryland, College Park - MSE, CNAM

  • I. Takeuchi

    Department of Materials Science and Engineering, University of Maryland, College Park, MD 20424, University of Maryland, College Park - MSE, CNAM, Deparment of Materials Science and Engineering, University of Maryland, College Park, MD 20424

  • Kui Jin

    University of Maryland, Center for Nanophysics \& Advanced Materials, Department of Physics, University of Maryland, College Park, University of Maryland, College Park - Physics, CNAM

  • Richard Greene

    University of Maryland, College Park - Physics, CNAM