Disorder Induced Melting of Charge Density Wave Order in doped 2H-NbSe2 systems

ORAL

Abstract

Using a combination of Angle Resolved Photoemission Spectroscopy (ARPES), X-ray diffraction, transport and Scanning Tunneling Microscopy (STM) measurements on pristine as well as disordered 2H-NbSe2 samples, we have found that the onset Temperature Tcdw for Long Ranged Charge Density Wave (CDW) order gets quickly suppressed with concentration of disorder ions (X) and at certain critical concentration (Xc) it undergoes a quantum melting. Our STM measurements provide the evidence for local CDW ordering in doped samples for temperatures way above Tcdw. On the other hand, our ARPES measurements have found evidences for the presence of energy gap for both T$>$Tcdw {\&} X$>$Xc. We argue, all these experimental observations from completely different probes hint towards phase fluctuations of the order parameter as the mechanism behind the destruction of CDW order in quasi 2-d systems, such as 2H-NbSe2.

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Authors

  • Utpal Chatterjee

    Argonne National Laboratory, Argonne National Lab

  • Stephan Rosenkranz

    Argonne National Laboratory

  • J.-P. Castellan

    Argonne National Laboratory

  • Jasper van Wezel

    Argonne National Laboratory

  • Ray Osborn

    Argonne National Laboratory

  • Maria Iavarone

    Physics Department, Temple University, Philadelphia, PA 19122 USA, Temple University, Physics Department, Temple University, Philadelphia, PA 19122, USA

  • Goran Karapetrov

    Physics Department, Drexel University, Philadelphia, PA 19104 USA, Physics Department, Drexel University, Drexel University, Physics Department, Drexel University, Philadelphia PA 19104, USA, Department of Physics, Drexel University and Institute of Electrical Engineering, Slovak Academy of Sciences