Investigation of the role of spin-texture on the Na0.46CoO2

ORAL

Abstract

We will present magnetotransport properties and their relationship to a possible chiral spin texture in ultra-thin Na$_{0.46}$CoO$_{2}$ devices in high magnetic fields. This composition exhibits a weakly insulating state, with a frustrated local spin texture, unique, among the hexagonal Na$_{x}$CoO$_{2}$ family. Previous a large large Hall effect was found for composition $x$=0.5 (M. Foo \textit{et al.}, Phys. Rev. Lett. 92, 247001 (2004)) and prior high-field studies (L. Balicas \textit{et al.}, Phys. Rev. Lett. 94, 236402 (2005).) have found the existence of a small Fermi surface in the system and a two-fold angular magnetoresistance. To date however, the Hall-conductivity has not been investigated in magnetic fields strong enough to suppress the charge-order, above 41~T. Herein, we investigate the role of local spin-texture (in the charge-ordered state) on the Hall conductance by measuring both bulk and devices with only several monolayers thick in strong magnetic fields. Our investigations under magnetic fields ($B<$60 T) show that the high resistivity charge-order region is suppressed with out-of-plane field at $B\sim $41 T with highly non-monotonic -\textit{$\rho $}$_{xy}$ with a maximum at $B\sim $27 T and rapidly decreases to zero. However, magnetization measurements show no significant features within measurement accuracy indicating that magnetization changes are small at the field-induced phase transition. Recent theoretical advances suggest that this compound exhibits a quantum Hall state coupled with spin chirality (I. Martin, C. D. Batista, Phys. Rev. Lett. 101, 156402 (2008)).

Authors

  • J.W. Kim

    LANL

  • E.-D. Mun

    LANL

  • R. McDonald

    MPA-NHMFL, Los Alamos National Laboratory, Los Alamos, NM 87545, LANL

  • J.D. Thompson

    LANL, Los Alamos National Lab, Los Alamos National Laboratory

  • Ivar Martin

    LANL

  • C. Batista

    Theoretical Division, Los Alamos National Laboratory, Theoretical division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, LANL

  • Vivien Zapf

    Los Alamos National Laboratory, LANL, Los Alamos National Laboratory, Los Alamos, NM, Los Alamos National Lab

  • P. Moll

    Laboratory for Solid State Physics, ETH Zurich, Switzerland, ETH-Zurich

  • A. Morpurgo

    DPMC - University of Geneva, University of Geneva

  • D. Argyriou

    Helmholtz-Zentrum Berlin f\&#034;ur Materialien und Energie