RIXS Studies of Magnetic Excitations in Layered Iridates

COFFEE_KLATCH · Invited

Abstract

5$d$ Transition metal oxides lie at the intersection of strong spin-orbit coupling and electron correlation, and open a new playground for novel electronic phases with unconventional magnetic, superconducting, magneto-electric, and band-topological properties. In particular, a rich variety of magnetic phases are predicted from the magnetic interactions that take various forms ranging from Heisenberg to bond-directional dipolar-like couplings in the strong spin-orbit coupling limit. In this talk, I will review on these novel aspects of magnetism in iridates studied using resonant x-ray scattering techniques. Specifically, following topics will be discussed: (i) Heisenberg-like nature of magnetic coupling in Sr$_{2}$IrO$_{4}$ that sharply contrast with the unusually large spin-wave gap in Sr$_{3}$Ir$_{2}$O$_{7}$, (ii) the origin of strong Ising anisotropy in Sr$_{3}$Ir$_{2}$O$_{7}$, and (iii) the contrasting dynamics of ``spin-orbit exciton'' modes in the Heisenberg and Ising magnets.

Authors

  • B.J. Kim

    Materials Science Division, Argonne National Laboratory