Superconductivity in Nb$_3$Pd$_{0.75}$Se$_7$

ORAL

Abstract

Here, we report the discovery of superconductivity in the transition metal chalcogenide Nb$_3$Pd$_{0.75}$S$_7$ with a transition temperature $T_c = 1.9 $ K. In extremely thin, needle like single crystals we observe upper critical fields $H_{c2}^b(T \rightarrow 0$ K) $\simeq 14 $ T for fields directed along the needle axis, or the crystallographic \emph{b}-axis. This value is 4 times larger than the expected weak coupling Pauli limiting field. For fields applied along two directions perpendicular to the \emph{b}-axis, we observe considerably smaller but anisotropic upper critical fields. For fields along and perpendicular to the $b$-axis we observe a temperature-dependent anisotropy $\gamma = H_{c2}^b/H_{c2}^{\perp b}$ as large as 6 (as $T \rightarrow T_c$). This behavior suggests that this compound is a multi-band superconductor. The low symmetry of its crystallographic structure implying low electronic dimensionality, coupled to multi-band behavior and very high upper critical fields, suggests an unconventional superconducting ground-state.

Authors

  • Daniel Rhodes

    National High Magneti Field Lab, National High Magnetic Field Lab

  • Qiu Zhang

    National High Magnetic Field Laboratory, Tallahassee, FL, USA, National High Magneti Field Lab, National High Magnetic Field Lab

  • Bin Zheng

    National High Magneti Field Lab, National High Magnetic Field Lab

  • Gang Li

    Physics Dept., Univ. of Michigan, National High Magneti Field Lab, National High Magnetic Field Lab

  • Andhika Kiswandhi

    National High Magneti Field Lab

  • Tiglet Besara

    National High Magneti Field Lab

  • Theo Siegrist

    National High Magneti Field Lab

  • L. Balicas

    National High Magnetic Field Laboratory, Florida State University, Tallahassee, FL, USA, National High Magnetic Field Lab, Tallahassee, FL, Florida State University, National High Magneti Field Lab, National High Magnetic Field Lab, NHMFL