Superconductivity in Nb$_3$Pd$_{0.75}$Se$_7$

ORAL

Abstract

Here, we report the discovery of superconductivity in the transition metal chalcogenide Nb$_3$Pd$_{0.75}$S$_7$ with a transition temperature $T_c = 1.9 $ K. In extremely thin, needle like single crystals we observe upper critical fields $H_{c2}^b(T \rightarrow 0$ K) $\simeq 14 $ T for fields directed along the needle axis, or the crystallographic \emph{b}-axis. This value is 4 times larger than the expected weak coupling Pauli limiting field. For fields applied along two directions perpendicular to the \emph{b}-axis, we observe considerably smaller but anisotropic upper critical fields. For fields along and perpendicular to the $b$-axis we observe a temperature-dependent anisotropy $\gamma = H_{c2}^b/H_{c2}^{\perp b}$ as large as 6 (as $T \rightarrow T_c$). This behavior suggests that this compound is a multi-band superconductor. The low symmetry of its crystallographic structure implying low electronic dimensionality, coupled to multi-band behavior and very high upper critical fields, suggests an unconventional superconducting ground-state.

Authors

  • Daniel Rhodes

    • National High Magneti Field Lab
    • National High Magnetic Field Lab
  • Qiu Zhang

    • National High Magnetic Field Laboratory, Tallahassee, FL, USA
    • National High Magneti Field Lab
    • National High Magnetic Field Lab
  • Bin Zheng

    • National High Magneti Field Lab
    • National High Magnetic Field Lab
  • Gang Li

    • Physics Dept., Univ. of Michigan
    • National High Magneti Field Lab
    • National High Magnetic Field Lab
  • Andhika Kiswandhi

    • National High Magneti Field Lab
  • Tiglet Besara

    • National High Magneti Field Lab
  • Theo Siegrist

    • National High Magneti Field Lab
  • L. Balicas

    • National High Magnetic Field Laboratory, Florida State University, Tallahassee, FL, USA
    • National High Magnetic Field Lab, Tallahassee, FL
    • Florida State University
    • National High Magneti Field Lab
    • National High Magnetic Field Lab
    • NHMFL