Magnetic structure of R$_{2}$CoGa$_{8}$ (R $=$ Gd, Tb and Dy) and evolution of the magnetic structures along the series of intermetallic compounds with R $=$ Gd - Tm

ORAL

Abstract

In this work we have determined the magnetic structure of R$_{2}$CoGa$_{8}$ (R $=$ Gd, Tb and Dy) intermetallic compounds using X-ray resonant magnetic scattering in order to study the evolution of the anisotropic magnetic properties along the series for R $=$ Gd-Tm. The three compounds have a commensurate antiferromagnetic structure with a magnetic propagation vector (1/2 1/2 1/2) with N\'{e}el temperatures of 21.0, 27.5 and 15.2 K for R $=$ Gd, Tb and Dy, respectively. The critical exponent $\beta$ obtained from the temperature dependence of the integrated intensity of the resonant magnetic peaks suggest a 3D magnetism for the three compounds. The energy line shapes at the L$_{2}$ and L$_{3}$ edges of the magnetic peaks for these compounds present a purely dipolar character as demonstrated by comparison to first principle calculations. Comparing the simulated and integrated intensities corrected for absorption, we conclude that the magnetic moment direction is in the \textit{ab}-plane for Gd$_{2}$CoGa$_{8}$ compound and parallel to the $c-$axis for the Tb$_{2}$CoGa$_{8}$ and Dy$_{2}$CoGa$_{8}$ compounds. This information is used to discuss the evolution of the magnetic structure of R$_{2}$CoGa$_{8}$ series for R $=$ Gd-Tm where both the direction of the ordered moment and the ordering temperature evolution along the series can be explained through the competition between the indirect Ruderman-Kittel- Kasuya-Yoshida exchange interaction and crystalline electric field effects.

Authors

  • Carlos Giles

    Argonne National Laboratory

  • Jose Renato Madergan

    Argonne National Laboratory

  • Cris Adriano

    University of Illinois at Chicago

  • Rafael Vescovi

    University of Campinas

  • Pascoal Pagliuso

    University of Campinas, Unicamp