Evolution of magnetic structure in the square lattice iridate Sr$_{2}$Ir$_{\mathrm{1-x}}$Rh$_{\mathrm{x}}$O$_{4}$
ORAL
Abstract
5$d$ based iridates have continuously provides a fertile playground for the studies of novel physics driven by spin-orbit interaction (SOI) that rigorously competes with other relevant energies, particularly the on-site Coulomb interaction U. Using single crystal neutron diffraction and polarized neutron scattering analysis, we have investigated the evolution of spin and crystal structures in the doped Sr$_{2}$Ir$_{\mathrm{1-x}}$Rh$_{\mathrm{x}}$O$_{4}$(0$\le $x$\le $0.20). The parent Sr$_{2}$IrO$_{\mathrm{4}}$ shows canted antiferromagnetic structure with spin lies in the basal plane. The spin orientation closely follows the rotation of the IrO$_{6}$ octahedra with total ordered moment of 0.21 $\mu_{\mathrm{B}}$/Ir. A small amount of Rh ions doped at the Ir sites drastically reduces the magnetic transition and modifies the spin configuration. The neutron scattering results provide experimental insights into the magnetic and crystal structure crucial to the understanding this prototype iridates.
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Authors
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Feng Ye
Oak Ridge National Lab
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Songxue Chi
Oak Ridge National Lab, Oak Ridge National Laboratory
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Masaaki Matsuda
Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak RIdge Natl Lab, Oak Ridge National Lab
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Xiaoping Wang
Oak Ridge National Lab
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Christina Hoffmann
Oak Ridge National Lab
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Bryan Chakoumakos
Oak Ridge National Lab
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Jaime Fernandez-Baca
Oak Ridge National Lab
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Tongfei Qi
Center for Advanced Materials and Department of Physics and Astronomy, University of Kentucky, University of Kentucky
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Gang Cao
Department of Physics and Astronomy, University of Kentucky, Lexington, Kentucky 40506-0055, Center for Advanced Materials, Department of Physics and Astronomy, University of Kentucky, University of Kentucky