Fermi surface collapse, gap, coherence: an ARPES study of the hybridization in Ce$_2$RhIn$_8$
ORAL
Abstract
The crossover of localized magnetic moments at high temperatures into itinerant states of heavy mass at low temperatures in some metals containing \emph{f} electrons, first addressed by Kondo, is a fundamental problem in condensed matter physics involving a temperature dependent hybridization between \emph{f} levels and conduction electrons (\emph{ce}). Here we present an extensive angular resolved photoemission spectroscopy study performed in Ce$_2$RhIn$_8$\ as a function of temperature. Our experiments reveal the presence of three energy scales, differing by an order of magnitude from each other: first at room temperature, where the \emph{f} levels are localized, we observe a small Fermi surface (FS), which undergoes dramatic topological changes toward a large FS near the minimum in the resistivity around 200K; the opening of a spectral gap below 30K without a change in topology of the Fermi surface; and finally, below 5K, composite quasiparticles form, as the resistivity suddenly decreases. The expectation that hybridization, spectral gap, and \emph{f} electron coherence go hand in hand should be expanded to include the possibility of separate energy scales for each of these phenomena.
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Authors
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Fanny Rodolakis
Argonne National Laboratory
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Cris Adriano
University of Campinas
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Francisco Restrepo
University of Illinois at Chicago
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Priscila Rosa
University of Campinas, Univ of California - Irvine, University of California at Irvine, Universidade Estadual de Campinas
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Pascoal Pagliuso
University of Campinas, Universidade Estadual de Campinas
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Juan Carlos Campuzano
University of Illinois at Chicago, Materials Science Division, Argonne National Laboratory and Dept. of Physics, University of Illinois, Chicago