Phonon spectrum of SrFe$_{2}$As$_{2}$ determined using multizone phonon refinement

ORAL

Abstract

The ferropnictide superconductors exhibit a sensitive interplay between the lattice and magnetic degrees of freedom, including a number of phonon modes are much softer than predicted by nonmagnetic calculations using density functional theory (DFT). However, it is not known what effect, if any, the long-range magnetic order has on phonon frequencies above 23~meV, where several phonon branches are very closely spaced in energy and it is challenging to isolate them from each other. We measured these phonons using inelastic time-of-flight neutron scattering in $\approx$ 40~Brillouin zones, and developed a technique to determine their frequencies. We find this method capable of determining phonon energies to better than 0.1~meV accuracy, and that the DFT calculations using the experimental structure yield qualitatively correct energies and eigenvectors. We do not find any effect of the magnetic transition on these phonons.

Authors

  • D. Parshall

    Univ of Colorado, Boulder

  • R. Heid

    Karlsruhe Institute of Technology

  • J.L. Niedziela

    Oak Ridge National Laboratory, Instrument and Source Division, Oak Ridge National Laboratory

  • Thomas Wolf

    Karlsruhe Institute of Technology, Karlsruher Institut f\"ur Technologie, IFP, 76021 Karlsruhe, Germany

  • M.B. Stone

    Oak Ridge National Laboratory

  • D.L. Abernathy

    Oak Ridge National Laboratory, Oak Ridge National Lab, Quantum Condensed Matter Division, Oak Ridge National Laboratory

  • Dmitry Reznik

    Univ of Colorado, Boulder, Department of Physics, University of Colorado-Boulder