Phonon spectrum of SrFe$_{2}$As$_{2}$ determined using multizone phonon refinement
ORAL
Abstract
The ferropnictide superconductors exhibit a sensitive interplay between the lattice and magnetic degrees of freedom, including a number of phonon modes are much softer than predicted by nonmagnetic calculations using density functional theory (DFT). However, it is not known what effect, if any, the long-range magnetic order has on phonon frequencies above 23~meV, where several phonon branches are very closely spaced in energy and it is challenging to isolate them from each other. We measured these phonons using inelastic time-of-flight neutron scattering in $\approx$ 40~Brillouin zones, and developed a technique to determine their frequencies. We find this method capable of determining phonon energies to better than 0.1~meV accuracy, and that the DFT calculations using the experimental structure yield qualitatively correct energies and eigenvectors. We do not find any effect of the magnetic transition on these phonons.
–
Authors
-
D. Parshall
Univ of Colorado, Boulder
-
R. Heid
Karlsruhe Institute of Technology
-
J.L. Niedziela
Oak Ridge National Laboratory, Instrument and Source Division, Oak Ridge National Laboratory
-
Thomas Wolf
Karlsruhe Institute of Technology, Karlsruher Institut f\"ur Technologie, IFP, 76021 Karlsruhe, Germany
-
M.B. Stone
Oak Ridge National Laboratory
-
D.L. Abernathy
Oak Ridge National Laboratory, Oak Ridge National Lab, Quantum Condensed Matter Division, Oak Ridge National Laboratory
-
Dmitry Reznik
Univ of Colorado, Boulder, Department of Physics, University of Colorado-Boulder