Spin-orbital separation in the anisotropic ladder system CaCu$_2$O$_3$

ORAL

Abstract

Recently, resonant inelastic X-ray scattering (RIXS) on the 1D spin system Sr$_2$CuO$_3$ has revealed an unprecedented dispersion of orbital excitations [Nature 485, 82 (2012)]. This result has been interpreted as the fractionalization of spin and orbital degree of freedom from the elementary electron, hallmark of one dimensional physics as the previously observed spin-charge separation [Nature Phys. 2, 397 (2006)]. How these phenomena carry over into higher dimensions remains currently unclear. To clarify this point, we studied the spin and orbital excitations of the anisotropic ladder CaCu$_2$O$_3$, which realizes a first step towards 2D correlated electron systems. Combining high-resolution RIXS experiments with theoretical model calculations we show that spin-orbital fractionalization indeed occurs in CaCu$_2$O$_3$ and prevails beyond the strict 1D limit [arXiv:1310.8346]. We also establish that such a fractionalization is far more robust than the spin-charge separation. The main reasons behind this are the intrinsic 1D orbital dynamics and the fact that the spinons are faster than the orbitons but slower than the holons.

Authors

  • Valentina Bisogni

    Paul Scherrer Institut, Villigen PSI, Switzerland

  • Krzysztof Wohlfeld

    SLAC National Laboratory and Stanford University, Menlo Park, USA

  • Satoshi Nishimoto

    IFW Dresden, Germany

  • Claude Monney

    Fritz-Haber-Insitut, Berlin, Germany

  • Jan Trinckauf

    IFW Dresden, Germany

  • Kejin Zhou

    Diamond Light Source , Didcot, UK

  • Roberto Kraus

    IFW Dresden, Germany

  • Thorsten Schmitt

    Paul Scherrer Institut, Villigen PSI, Switzerland

  • Jeroen van den Brink

    IFW Dresden, Germany, Institute for Theoretical Solid State Physics, IFW Dresden, Helmholtzstr. 20, 01069 Dresden, Germany, Institute for Theoretical Solid State Physics, IFW Dresden, Germany

  • Jochen Geck

    IFW Dresden, Germany, Institute for Solid State Research, IFW Dresden, Germany