Lensless imaging of atomic surface structures using ptychography in reflection mode

ORAL

Abstract

We propose that atomic structures on single crystal surfaces can be imaged using a variation of coherent x-ray diffractive imaging. This is a lensless ptychographic technique applied along the crystal truncation rod in reciprocal space. Simulations show that the highest sensitivity on the monolayer surface structure is obtained at the anti-Bragg condition. We demonstrate the feasibility of ptychographic reconstruction from experimental data collected in reflection mode by reconstruction of atomic steps on a crystal surface. This work and use of the Advanced Photon Source and the Electron Microscopy Center for Materials Research were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The work at Safarik University is supported by Slovak grant VEGA 1/0782/12 and ERDF EU grant under contract No. ITMS 26220120005

Authors

  • Chenhui Zhu

    Argonne National Lab

  • Ross Harder

    Argonne National Lab, APS-Argonne National Lab

  • Ana Diaz

    Paul Scherrer Institut, Switzerland

  • Vladimir Komanicky

    Safarik University, Slovakia, Safarik University - Department of Condensed Matter Physics

  • Andi Barbour

    Argonne National Lab, Argonne National Laboratory - Material Science Division

  • Ruqing Xu

    Argonne National Lab

  • Xiaojing Huang

    Brookhaven National Lab

  • Yaohua Liu

    Argonne National Lab, Argonne National Laboratory, Materials Science Division, Argonne National Laboratory

  • Michael Pierce

    Rochester Institute of Technology, Rochester Inst of Tech, Rochester Institute of Technology - School of Physics and Astronomy

  • Hoydoo You

    Argonne National Lab, Argonne National Laboratory - Material Science Division