Magnetic Texture {\&} Frustration in Quantum Magnets via Strain Measurements to 100 Tesla

COFFEE_KLATCH · Invited

Abstract

Strong geometrical frustration in magnets leads to exotic states, such as spin liquids, spin supersolids, magnetic solitons, and complex magnetic textures. SrCu$_{2}$(BO$_{3})_{2}$, a spin-1/2 Heisenberg antiferromagnet in the archetypical Shastry-Sutherland lattice, exhibits a rich spectrum of magnetization plateaus and stripe-like magnetic textures in applied fields. We observed new magnetic textures via optical FBG magnetostriction and magnetocaloric measurements in fields up to 100.75 Tesla at 73.6 T and at 82 T [1] which we attribute, using a controlled density matrix renormalization group approach, to a 2/5 plateau and to the long-predicted 1/2-saturation plateau. The plateau predicted at 2/5 saturation is particularly interesting since strain appears to be the only experimental probe with enough sensitivity to reveal it as magnetization probes see a much more gradual change in the same field range [2,3]. BiCu$_{2}$PO$_{6}$ is a frustrated two-leg spin ladder compound with a spin gap that can be closed with a magnetic field of approximately 20T to induce a soliton lattice [4,5]. Time permitting, I will also discuss magnetization, magnetostriction and specific heat vs magnetic fields to 65 T used to obtain the anisotropic (H,T) phase diagram in BiCu$_{2}$PO$_{6}$ single crystal samples. Work at the NHMFL was supported by the National Science Foundation, the US Department of Energy Office of Basic Energy Science through the project ``Science at 100 Tesla,'' and the State of Florida.\\[4pt] [1] M. Jaime, et al. \textit{Proc. Natl. Acad. Sci.} \textbf{109}, 12407 (2012).\\[0pt] [2] S.E. Sebastian, et al., \textit{Proc. Natl. Acad.} Sci. \textbf{105}, 20157 (2009).\\[0pt] [3] Y.H. Matsuda, et al., \textit{Phys. Rev. Lett.} \textbf{111}, 137204 (2013).\\[0pt] [4] Y. Kohama, et al., Phys. Rev. Lett. \textbf{109}, 167204 (2012). \\[0pt] [5] F. Cassola, et al., Phys. Rev. Lett. \textbf{110}, 187201 (2013).

Authors

  • Marcelo Jaime

    NHMFL-LANL, Los Alamos, NM 87544