Magnetic fluctuations induced insulator-to-metal transition in Ca(Ir$_{\mathrm{x}}$Ru$_{\mathrm{1-x}})$O$_{3}$

ORAL

Abstract

The Fermi liquid theory dictates the metal-insulator transition in a continuous fashion via the divergence of the quasiparticle mass m*. However, the metallic phase near the Mott insulator in the metal-insulator phase diagram based on the Hubbard model is dominated by the fluctuations of spin, charge and orbital correlations; often termed as the anomalous metallic phase. In this presentation, experimental results manifesting the magnetic fluctuations induced insulator-to-metal transition in Ca(Ir$_{\mathrm{x}}$Ru$_{\mathrm{1-x}})$O$_{3}$ will be discussed in the framework of the Hubbard model. For x $=$ 1, the compound CaIrO$_{3}$ is a Mott insulator with antiferromagnetic order below T $\sim$ 110 K. A gradual substitution of Ir by Ru results in the onset of anomalous metallic behavior as a function of the tuning parameter x. At x $=$ 0, the compound CaRuO$_{3}$ is a non-Fermi liquid metal with no apparent magnetic order. While the orthorhombic structural integrity is maintained throughout the group, strong magnetic fluctuations is detected below x $=$ 0.8. The role of magnetic fluctuations in the metallic transition is further confirmed by first principle theoretical calculation.

Authors

  • Deepak Singh

    Univ of Missouri - Columbia, University of Missouri, Columbia

  • Jagath Gunasekera

    University of Missouri, Columbia

  • Ashutosh Dahal

    University of Missouri, Columbia

  • Leland Harriger

    NIST, National Institute of Standards and Technology, Gaithersburg

  • Thomas Heitmann

    University of Missouri, MURR, University of Missouri Research Reactor, Columbia