Photocatalytic Solar Fuel Generation on Semiconductor Nanocrystals
COFFEE_KLATCH · Invited
Abstract
I will review our scientific work on photocatalytic solar fuel generation utilizing colloidal semiconductor nanocrystals decorated with catalytic metal clusters. In particular, nanocrystals made of CdS, TiO$_{2}$ and organo-metal halide perovskites will be discussed. Key issues are the role of hole scavangers (M. Berr et al., Appl. Phys. Lett. 100, 223903 (2012)), the size and density of catalytic clusters (M. Berr et al.: Appl. Phys. Lett. 97, 093108 (2010) and Nano Letters 12, 5903 (2012) , and dependencies on external parameters such as pH (T. Simon et al., Nature Mat. 13, 1013 (2014)).
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Authors
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Jochen Feldmann
Photonics and Optoelectronics Group, Ludwig-Maximilians-Universitaet (LMU), Munich, Germany