CF excitations of CeCu$_2$Si$_2$: Revisited employing a single crystal and triple-axis spectrometers

ORAL

Abstract

CeCu$_2$Si$_2$ is the famous heavy-fermion system showing unconventional superconductivity mediated by low-energy magnetic excitations of the CF ground-state doublet. From the point symmetry of the Ce$^{3+}$ ions in the tetragonal crystal lattice a CF splitting into 3 doublets is expected for the (J=5/2) multiplet. First INS measurements on polycrystalline samples of CeCu$_2$Si$_2$ employing a time-of-flight technique revealed a CF level scheme of 0-12-30 meV but were disputed by more advanced INS data in subsequent years. Finally it was accepted that the CF excitations of CeCu$_2$Si$_2$ consist of only one very broad transition with 30 meV from the ground-state doublet to both of the more or less degenerated excited CF states, the so called ``quasi-quartet.'' Employing a large single crystal of CeCu$_2$Si$_2$ and the thermal neutron triple-axis spectrometers PUMA at FRM II and TAIPAN at OPAL we revisited the CF-transitions to verify or falsify this interpretation. We performed TAS measurements for different crystallographic directions. From our results we infer that the quasi-quartet actually consists of two doublets situated at 30 and 35 meV exhibiting a strong directional dependence of their transition matrix elements to the ground state doublet.

Authors

  • Michael Loewenhaupt

    Tech Univ Dresden

  • Sergey Danilkin

    ANSTO

  • Guochu Deng

    ANSTO

  • Klaudia Hradil

    TU Wien

  • Oliver Stockert

    MPI-CPfS

  • Astrid Schneidewind

    JCNS-MLZ