Electronic and magnetic properties of (1 1 1)-oriented CoCr$_2$O$_4$ epitaxial thin film

ORAL

Abstract

We report on the fabrication of high quality (1 1 1)-oriented ferrimagnetic normal spinel CoCr$_2$O$_4$ epitaxial thin films on single crystal Al$_2$O$_3$ substrates. The structural, electronic and magnetic properties were characterized by $in$-$situ$ reflection high energy electron diffraction, atomic force microscopy, X-ray diffraction, X-ray photoemission spectroscopy, SQUID magnetometry and element resolved resonant X-ray magnetic scattering. The comprehensive characterization reveals that no disorder in the cation distribution or multivalency issue is present in the samples. As a result, Kagom\'e and triangular layers are naturally formed via this specific growth approach. These findings offer a pathway to fabricate two dimensional Kagom\'e heterostructures with novel quantum many-body phenomena by means of geometrical design.

Authors

  • Xiaoran Liu

    Department of Physics, University of Arkansas

  • Mikhail Kareev

    Department of Physics, University of Arkansas, Univ of Arkansas-Fayetteville

  • Yanwei Cao

    Department of Physics, University of Arkansas, University of Arkansas

  • Jian Liu

    University of California, Berkeley, Department of Physics, University of California, Berkeley

  • Srimanta Middey

    Department of Physics, University of Arkansas

  • Derek Meyers

    University of Arkansas, Department of Physics, University of Arkansas

  • John Freeland

    Advanced Photon Source, Argonne National Laboratory, Argonne National Laboratory, Advanced Photon Source, Argonne National Lab, Argonne, IL

  • Jack Chakhalian

    Department of Physics, University of Arkansas, University of Arkansas