\textbf{Wall-like spin excitations in A-type antiferromagnetic CaCo}$_{\mathrm{\mathbf{2}}}$\textbf{As}$_{\mathrm{\mathbf{2}}}$

ORAL

Abstract

The $A$Co$_{\mathrm{2}}$As$_{\mathrm{2\thinspace }}(A =$ Ca, Sr, Ba ) compounds are structurally and chemically similar to $A$Fe$_{\mathrm{2}}$As$_{\mathrm{2\thinspace }}$and possess some interesting similarities and differences in their magnetism. We recently discovered that SrCo$_{\mathrm{2}}$As$_{\mathrm{2}}$ has stripe antiferromagnetic (AFM) spin correlations similar to stripe-ordered $A$Fe$_{\mathrm{2}}$As$_{\mathrm{2}}$. On the other hand, CaCo$_{\mathrm{2}}$As$_{\mathrm{2}}$ orders in an A-type AFM structure with ferromagnetic correlation of the spins in the square-lattice Co-layer and AFM correlations between layers. Despite the A-type order, our recent inelastic neutron scattering measurements show that spin excitations in CaCo$_{\mathrm{2}}$As$_{\mathrm{2}}$ are not associated with either the A-type or stripe-type order. Instead, we observe broad excitations that extend longitudinally (along (1,1,0) in reciprocal space), but remain sharply defined in the transverse direction. These excitations seem to be best characterized as a ``wall'' of scattering and suggest that CaCo$_{\mathrm{2}}$As$_{\mathrm{2}}$ has quasi-one-dimensional spin dynamics very different than in $A$Fe$_{\mathrm{2}}$As$_{\mathrm{2}}$ and SrCo$_{\mathrm{2}}$As$_{\mathrm{2}}$.

Authors

  • A. Sapkota

    Ames Lab., Dept. of Physics and Astronomy, Iowa State Univ., Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University, Ames Lab. & Iowa State Univ., Ames, IA, 50011

  • B. G. Ueland

    Ames National Laboratory, Ames Lab., Dept. of Physics and Astronomy, Iowa State Univ., Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University

  • A. Pandey

    Ames Lab., Dept. of Physics and Astronomy, Iowa State Univ., Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University, Ames Laboratory, Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Ames Lab. & Iowa State Univ., Ames, IA, 50011

  • David C. Johnston

    Ames Lab., Dept. of Physics and Astronomy, Iowa State Univ., Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University, Ames Laboratory, Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Ames Lab. & Iowa State Univ., Ames, IA, 50011, Iowa State Univ, Ames Laboratory, Dept. of Phys. and Astro, Iowa State Univ.

  • A. Kreyssig$^{*}$

    Ames Laboratory, U.S. DOE and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA, Ames Lab., Dept. of Physics and Astronomy, Iowa State Univ., Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University, Ames Lab. & Iowa State Univ., Ames, IA, 50011, $^*$Ames Laboratory, Dept. of Phys. and Astro., Iowa State University, IA, USA; $^+$University of Missouri Research Reactor, MO, USA

  • R.J. McQueeney

    Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University, Ames Lab. & Iowa State Univ., Ames, IA, 50011

  • Alan Goldman

    Ames Laboratory, U.S. DOE and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA, Ames Lab., Dept. of Physics and Astronomy, Iowa State Univ., Ames Laboratory, Dept. of Physics and Astronomy, Iowa State University, Ames Lab. & Iowa State Univ., Ames, IA, 50011, Iowa State University

  • V. K. Anand

    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH

  • Jennifer L. Niedziela

    Oak Ridge National Laboratory, Oak Ridge NAtional Lab., TN, 37831, Oak Ridge National Laboratory, Materials Science Division

  • Douglas Abernathy

    Oak Ridge National Laboratory, Oak Ridge NAtional Lab., TN, 37831