Quasi-Elastic Neutron Scattering Study of Characteristic Features of Water Dynamics in Confined Geometries

ORAL

Abstract

Water trapped in restricted environments is ubiquitous in nature and known to influence many biochemical and geophysical processes. Understanding the structural and dynamical properties of nano-confined water (very different than those of the bulk phase) is thus of key fundamental interests. We present a survey of various quasi-elastic neutron (QENS) studies of nano-confined water, which we further analyzed in the context of a proposed universal scaling law. Using this predictive law, we specifically investigate how the diffusive behavior of water changes with changing hydration level, confinement size, or geometry. Finally, we present our recent QENS results of water in nanoporous media evaluated using this scaling law.

Authors

  • Souleymane Diallo

    Oak Ridge National Laboratory Oak Ridge, TN, USA, Oak Ridge National Laboratory, Oak Ridge National Lab

  • Naresh Osti

    Oak Ridge National Laboratory, Oak Ridge, TN, USA

  • Alexandra Cote

    University of Miami, FL, USA

  • Eugene Mamontov

    Oak Ridge National Laboratory, Oak Ridge, TN, USA, Oak Ridge National Lab

  • Anibal Ramirez-Cuesta

    Oak Ridge National Laboratory, Oak Ridge, TN, USA

  • David Wesolowski

    Oak Ridge National Laboratory, Oak Ridge, TN, USA