Magnetism and structure of a half-metallic Heusler compound Co-Mn-Cr-Si

Half metallic ferromagnetic Heusler compounds have a potential in the development of spintronic devices for its high spin polarization at the Fermi level and lattice structure compatibility. Heusler compounds based on cobalt are considered a good candidate for room temperature half-metals due to their high Curie temperature. Co$_{\mathrm{2}}$CrSi is one of such predicted half-metal, but it is meta-stable and difficult to synthesize in the desired crystal structure. We have successfully synthesized a Heusler compound Co$_{\mathrm{2}}$Mn$_{\mathrm{0.5}}$Cr$_{\mathrm{0.5}}$Si by using arc melting and rapid quenching followed by thermal treatment under high vacuum to control any parasitic contamination. Crystal X-ray diffraction pattern shows the samples crystallize in a cubic Heusler structure with some degrees of structural disorder. Curie temperatures of the prepared samples are observed well beyond room temperature near 900 K. Magnetic anomalies present in as-prepared samples are cleared, and its magnetic properties are improved by thermal treatment.