High field fermiology of the metallized Mott insulator NiS$_2$

ORAL

Abstract

Long a prominent theme in the physics of strongly correlated electron systems, the Mott metal-to-insulator transition continues to be an active topic of investigation; various mechanisms have been proposed for the formation of the Mott insulating state, but its precise nature remains an open question. In many such systems under study, filling (via chemical doping) is used as a tuning parameter, but the resultant disorder hinders the use of sensitive quantum oscillation techniques to study Fermi surface properties. In the prototypical Mott insulator NiS$_2$, one can instead use pressure to cleanly tune the ratio $U/t$ of onsite Coulomb repulsion to kinetic energy across the phase diagram. We will present our recent quantum oscillation measurements of NiS$_2$ under hydrostatic pressures from near the Mott transition up to 55 kbar, comparing the evolution of the Fermi surface and effective masses upon approaching the Mott transition to expectations from DFT calculations. We observe a large Fermi surface persisting to the transition along with a divergent effective mass, consistent with a Brinkman-Rice picture.

Authors

  • Jordan Baglo

    Cavendish Laboratory, University of Cambridge

  • Hui Chang

    Cavendish Laboratory, University of Cambridge

  • Konstantin Semeniuk

    Cavendish Laboratory, University of Cambridge

  • Xiaoye Chen

    Cavendish Laboratory, University of Cambridge

  • Pascal Reiss

    Clarendon Laboratory, University of Oxford, UK, Cavendish Laboratory, University of Cambridge

  • Hong En Tan

    Cavendish Laboratory, University of Cambridge

  • Patricia Alireza

    Cavendish Laboratory, University of Cambridge

  • Alix McCollam

    HFML, Nijmegen

  • Inge Leermakers

    HFML, Nijmegen

  • Sven Friedemann

    University of Bristol, H. H. Wills Laboratory, University of Bristol

  • Monika Gamza

    Jeremiah Horrocks Institute, University of Central Lancashire

  • Audrey Grockowiak

    NHMFL, Tallahassee, Florida, National High Magnetic Field Laboratory, NHMFL

  • William Coniglio

    NHMFL, Tallahassee, Florida, National High Magnetic Field Laboratory

  • Stan Tozer

    NHMFL, Tallahassee, Florida, National High Magnetic Field Laboratory

  • F. Malte Grosche

    Cavendish Laboratory, University of Cambridge