Thermal conductivity of actinide materials measured using the 3$\omega $ method

ORAL

Abstract

The thermal conductivity of nuclear materials governs the conversion of heat produced from fission events into electricity and it is an important parameter in reactor design and safety.~However, it is also a challenging property to measure due to radioactivity and radiotixicity of actinides. Most of the conventional methods require usage of large samples (millimeter size at least) with an appropriate shape. The 3$\omega $-method, developed by Cahill [D. G. Cahill,~\textit{Review of Scientific Instruments},~61, 802 (1990)], is designed to work with small samples and enables to measure thermal conductivity and heat capacity of bulk and thin layered materials. In this work, we have adapted the 3$\omega $~method to measure thermal conductivity and heat capacity of various metallic and insulating samples including small single crystals of UO$_{\mathrm{2}}$~and UN. The validity of this method has been also tested by measuring thermal conductivities of several testing materials (Cu, Pt, Constantan, SiO$_{\mathrm{2}})$. The new measurement setup has been adapted to be compatible with Quantum Design PPMS system.

Authors

  • Keshav Shrestha

    Idaho National Laboratory

  • K. Gofryk

    Idaho National Laboratory, INL