A layered Dirac system candidate: Fermi surface and anomalous Berry phase in ZrSiSe

ORAL

Abstract

ZrSiSe was recently claimed to correspond to a novel type of nodal Dirac system. We synthesized single crystals through a combination of solid state reaction and chemical vapor transport. The as-grown single crystals display residual resistivities on the order of 100 nOhmcm at 2K yielding a resistivity ratio surpassing 200. Magnetoresistance (MR) measurements reveal a non-saturating increase in the resistivity by a factor of 500000{\%} under fields up to 35 Tesla. De Haas van Alphen measurements under high magneticfields reveal a Fermi surface that is more complex than previously reported, although its geometry generally agrees with band structure calculations that indicate Dirac-like dispersion in the bulk around the Fermi energy. The charge carrier effective masses extracted from Lifshitz-Kosevich (LK) fits to the amplitude of quantum oscillations were found to range between 0.08me to 0.5me where me is the free electron mass. Fittings of the oscillatory signal to the LK formalism further reveal the existence of cyclotron orbits displaying non-trivial Berry phases approaching pi, which is consistent with the expectations from band structure calculations.

Authors

  • Yu-Che Chiu

    NHMFL and FSU, Department of Physics, Florida State University

  • Kuan-wen Chen

    NHMFL and FSU, National High Magnetic Field Lab,Tallahassee

  • David Graf

    National High Magnetic Field Laboratory, NHMFL, National High Magnetic Field Laboratory., National High Magnetic Field Laboratory Tallahassee, Florida State University, National High Magnetic Field Lab,Tallahassee

  • Qiong Zhou

    National High Magnetic Field Laboratory and Florida State University, NHMFL-FSU, NHMFL and FSU

  • Thomas J. Martin

    Department of Chemistry and Biochemistry, University of Texas at Dallas

  • Julia Chan

    UT-Dallas, Department of Chemistry and Biochemistry, University of Texas at Dallas, University of Texas at Dallas, Department of Chemistry and Biochemistry, The University of Texas at Dallas

  • Michelle Johannes

    Center for Computational Materials Science, Navel Research Laboratory

  • Ryan Baumbach

    NHMFL, National High Magnetic Field Laboratory, Florida State University, National High Magnetic Field Lab,Tallahassee

  • Luis Balicas

    NHMFL-FSU, NHMFL, National High Magnetic Field Lab, Natl High Magnetic Field Lab, Tallahassee, FL, USA