Dynamical criticality in high-dimensional glass-forming liquids.

ORAL

Abstract

The mean-field theory of glass formation predicts the existence of a dynamical critical point at which the relaxation time diverges. Due to the presence of activated processes in physical dimensions (d=2, 3), this critical point is then but a crossover. Some of the associated phenomenology is nonetheless considered to persist. We here aim to identify what, if anything, of this criticality can be clearly identified by systematically varying the dimension of space. Using fluids of polydispersed hard spheres that have been optimized for the swap Monte Carlo algorithm allows us to thermalize very high-density systems and thus to approach the regime of interest easily. We then examine markers of dynamical criticality, such as the fluctuations of dynamical correlators and dynamical heterogeneity.

Presenters

  • Patrick Charbonneau

    Duke University, Chemistry, Duke University, Department of Chemistry, Duke Univ, Duke Univ, Chemistry and Physics, Duke University

Authors

  • Ludovic Berthier

    Laboratoire Charles Coulomb, CNRS, Laboratoire Charles Coulomb, UMR 5221 CNRS, Université de Montpellier, Laboratoire Charles Coulomb, Université de Montpellier and CNRS, Laboratoire Charles-Coulomb, Université de Montpellier

  • Patrick Charbonneau

    Duke University, Chemistry, Duke University, Department of Chemistry, Duke Univ, Duke Univ, Chemistry and Physics, Duke University

  • Silvio Franz

    Physique, Université Paris-Sud

  • Joyjit Kundu

    Duke Univ, Univ of California - Berkeley