Metallicity beyond Mott-Ioffe-Regel limit in n-doped strontium titanate
ORAL
Abstract
Cooling oxygen-deficient strontium titanate to liquid-helium temperature leads to a decrease in its electrical resistivity by several orders of magnitude. The temperature dependence of resistivity follows a T-cubic behavior before becoming quadratic in the low-temperature limit, as expected in a Fermi liquid. Here, we show that the roughly cubic resistivity above 100K corresponds to a regime where the quasi-particle mean-free-path is shorter than the electron wave-length and the interatomic distance. These criteria define the Mott-Ioffe-Regel limit. Exceeding this limit occurs in strontium titanate well below room temperature, in contrast to other perovskytes. We argue that the T-cubic resistivity cannot be accounted for by electron-phonon scattering à la Bloch-Gruneisen and consider an alternative scheme based on Landauer transmission between individual dopants hosting polarons. We find a scaling relationship between carrier mobility, the electric permittivity and the frequency of transverse optical soft mode in this temperature range. Providing an account of this observation emerges as a challenge to theory.
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Presenters
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Kamran Behnia
Laboratoire Physique et Etude de Matériaux (UMR 8213 CNRS-ESPCI), Laboratoire de Physique Et d’Etude des Matériaux (UPMC-CNRS), ESPCI Paris, 10 Rue Vauquelin, ESPCI, ESPCI, LPEM CNRS
Authors
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Kamran Behnia
Laboratoire Physique et Etude de Matériaux (UMR 8213 CNRS-ESPCI), Laboratoire de Physique Et d’Etude des Matériaux (UPMC-CNRS), ESPCI Paris, 10 Rue Vauquelin, ESPCI, ESPCI, LPEM CNRS
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Xiao Lin
Nanyang Technological University, 10 Rue Vauquelin, ESPCI
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Willem Rischau
Laboratoire Physique et Etude de Matériaux (UMR 8213 CNRS-ESPCI), 10 Rue Vauquelin, ESPCI, ESPCI, LPEM CNRS
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Benoit Fauque
Laboratoire Physique et Etude de Matériaux (UMR 8213 CNRS-ESPCI), 10 Rue Vauquelin, ESPCI, ESPCI, LPEM CNRS