Short range order in the quantum XXZ honeycomb lattice material γ-BaCo2(PO4)2

ORAL

Abstract

γ-BaCo2(PO4)2 (γ-BCPO) is a honeycomb-lattice compound with quasi-two-dimensional structure exhibiting short-range ordered (SRO) frustrated magnetism. We have studied hydrothermally synthesized γ-BCPO samples via magnetometry (Χac), specific heat (Cp), x ray and inelastic neutron scattering (INS) experiments. Χac and Cp showed a broad anomaly at ∼ 5 K, with two weak kink features in Cp at TN1 ∼ 6 K and TN2 ∼ 3.5 K. Collinear antiferromagnetic SRO with ordering wavevector |kc| = 0.5 and correlation length ξc = 60 Å and quasi-2D helical SRO with |kh| = 0.25 and ξh = 253 Å form below TN1 and TN2 respectively. Our INS data compares well with linear spin wave theory for two separate parameter regimes of the XXZ J1-J2-J3 model with near neighbor ferromagnetic exchange, J1. Competing further interactions, J2 and J3 place γ-BCPO near regions of high classical degeneracy such as the highly frustrated point, J1/2 = -J2 = J3. Our analysis suggests that γ-BCPO balances near the edge of competing classical phases of the XXZ J1-J2-J3 model, implying that frustration and quantum fluctuations may account for its inability to form a long range order state.

Presenters

  • Harikrishnan Nair

    Department of Physics, Univ of Texas at El Paso, Department of Physics, University of Texas at El Paso

Authors

  • Harikrishnan Nair

    Department of Physics, Univ of Texas at El Paso, Department of Physics, University of Texas at El Paso

  • Jesse Brown

    Department of Physics, Colorado State University

  • Ethan Coldren

    Department of Physics, Colorado State University

  • Gavin Hester

    Department of Physics, Colorado State University

  • Martin Gelfand

    Department of Physics, Colorado State University

  • Andrei Podlesnyak

    Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge National Lab, Oak Ridge National Laboratory

  • Kate Ross

    Physics, Colorado State University, Department of Physics, Colorado State University, Colorado State University