Local fluctuations in the relaxation rate in glassy systems: probing dynamical heterogeneity and its exchange time
ORAL
Abstract
We numerically study the equilibrium dynamics of a glass-forming binary hard-sphere mixture in three dimensions, for different packing fractions. We provide a quantitative description of dynamical heterogeneity in terms of fluctuations in the local relaxation rates. We extract a newly defined two-point correlator, χ2Φ(t), that probes those fluctuations. The time decay of χ2Φ(t) is characterized by a certain time scale τex, which we identify as the exchange time of the slow and fast regions. We calculate the exchange time τex as a function of packing fraction, and we find that in the vicinity of the glass transition, τex is an order of magnitude longer then the α-relaxation time, τα.
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Presenters
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Rajib Pandit
Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University
Authors
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Rajib Pandit
Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University
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Elijah Flenner
Department of Chemistry, Colorado State University, Chemistry, Colorado State University
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Horacio Castillo
Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University, Physics and Astronomy, Ohio University