Local fluctuations in the relaxation rate in glassy systems: probing dynamical heterogeneity and its exchange time

ORAL

Abstract

We numerically study the equilibrium dynamics of a glass-forming binary hard-sphere mixture in three dimensions, for different packing fractions. We provide a quantitative description of dynamical heterogeneity in terms of fluctuations in the local relaxation rates. We extract a newly defined two-point correlator, χ2Φ(t), that probes those fluctuations. The time decay of χ2Φ(t) is characterized by a certain time scale τex, which we identify as the exchange time of the slow and fast regions. We calculate the exchange time τex as a function of packing fraction, and we find that in the vicinity of the glass transition, τex is an order of magnitude longer then the α-relaxation time, τα.

Presenters

  • Rajib Pandit

    Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University

Authors

  • Rajib Pandit

    Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University

  • Elijah Flenner

    Department of Chemistry, Colorado State University, Chemistry, Colorado State University

  • Horacio Castillo

    Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University, Physics and Astronomy, Ohio University