Theory of nonequilibrium pump/probe electronic Raman scattering in strongly correlated materials

ORAL

Abstract

We employ nonequilibrium dynamical mean-field theory to solve for the nonresonant B1g response of a strongly correlated material after a large electric field pump. This electronic Raman scattering channel has no vertex corrections even in nonequilibrium. The problem can be exactly solved for the Falicov-Kimball model at half-filling, which exhibits a Mott metal-insulator transition. We describe what the response looks like for these nonequilibrium systems and show what features emerge due to the nonequilibrium nature of the experiment. Similar calculations can also be done for the A1g response, but they require vertex corrections.

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Presenters

  • James Freericks

    Department of Physics, Georgetown Univ, Georgetown University, Physics, Georgetown Univ, Department of Physics, Georgetown University

Authors

  • James Freericks

    Department of Physics, Georgetown Univ, Georgetown University, Physics, Georgetown Univ, Department of Physics, Georgetown University

  • Oleh Matveyev

    Institute of Condensed Matter Physics

  • Andrij Shvaika

    Institute of Condensed Matter Physics

  • Thomas Devereaux

    Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Stanford Univ, SLAC and Stanford University, SLAC National Accelerator Laboratory, SLAC - Natl Accelerator Lab, Stanford Institute for Materials and Energy Sciences, SLAC National Laboratory, Stanford University, SIMIS, Stanford University, Physics, Stanford University, SLAC National Lab and Stanford University, SIMES, SLAC and Stanford University