Disordered Ferromagnetic Quantum Critical Point in CePd2P2 with Pd → Ni substitution

ORAL

Abstract

We report an investigation of the structural, thermodynamic, and electrical transport properties of the chemical substitution series Ce(Pd1-xNix)2P2. Pd → Ni substitution results in (1) contraction of the unit cell volume, which tunes the relative strengths of the Kondo and RKKY interactions, and (2) the introduction of disorder through alloying. The ferromagnetic ordering temperature TC is monotonically suppressed with increasing x, resulting in a quantum phase transition near xcr ≈ 0.75. In this region there is a logarithmic divergence in the electronic component of the heat capacity divided by temperature that is comparable to that seen for similar Ce-based systems near antiferromagnetic quantum critical points: e.g., CeCu2Si2. Together with a sub-quadratic temperature dependence of the electrical resistivity, this suggests a breakdown of Fermi-liquid behavior as would be expected near a quantum critical point. This behavior is examined in the context of the Belitz-Kirkpatrick-Vojta (BKV) theory, where the disorder causes the electronic soft modes to be diffusive and, as a result, the phase transition remains second order down to zero temperature. Based on this, we suggest that this is a model system for understanding ferromagnetic quantum criticality in a disordered metal.

Presenters

  • You Lai

    FSU-NHMFL, National High Magnetic Field Laboratory/Florida State University, National High Magnetic Field Laboratory, Natl High Magnetic Field Lab, NHMFL at Florida State University, Florida State Univ

Authors

  • You Lai

    FSU-NHMFL, National High Magnetic Field Laboratory/Florida State University, National High Magnetic Field Laboratory, Natl High Magnetic Field Lab, NHMFL at Florida State University, Florida State Univ

  • William Nelson

    FSU-NHMFL, Natl High Magnetic Field Lab

  • Yu-Che Qiu

    FSU-NHMFL

  • Kevin Huang

    National High Magnetic Field Lab, Florida State University, NHMFL, Natl High Magnetic Field Lab, NHMFL at Florida State University, National HIgh Magnetic Field Lab at Florida State University, National High Magnetic Field Lab at Florida State University, State Key Laboratory of Surface Physics, Department of Physics, Fudan University

  • Wes Potter

    FSU

  • Luis Balicas

    Natl High Magnetic Field Lab, Nat. High Magn. Field Lab., Florida State University, FSU-NHMFL, National High Magnetic Field Lab, National High Magnetic Field Laboratory, Natl. High Magnetic Field Lab, Florida State University, High Field Magnet Lab, 1800 E. Paul Dirac Drive, National High Magnetic Field Laboratory, Natl High Magnetic Field Lab

  • David Graf

    NHMFL Tallahassee, NHMFL, National High Magnetic Field Lab, National High Magnetic Field Laboratory, National High Magnetic Field Laboratory/Florida State University, Natl High Magnetic Field Lab, NHMFL at Florida State University, Florida State University, National High Magnetic Field Laboratory, Florida State University, Condensed Matter Science, NHMFL

  • Thomas Albrecht-Schmitt

    FSU, Florida State University, Chemistry, Florida State University

  • Ryan Baumbach

    National High Magnetic Field Laboratory, Florida State University, National High Magnetic Field Lab, Florida State University, National High Magnetic Field Laboratory, NHMFL, National High Magnetic Field Laboratory/Florida State University, Natl High Magnetic Field Lab, NHMFL at Florida State University