Quantum Spin Liquids Unveil the Genuine Mott State

ORAL

Abstract

The Widom line identifies the supercritical crossover from a gas-like to a more liquid-like behavior. A similar transition exists in correlated electron liquids, where the interplay of Coulomb repulsion, bandwidth and temperature triggers between the Mott insulating state and an incoherent conduction regime. Here we explore the electrodynamic response of three organic quantum spin liquids, where the absence of magnetic order enables unique insight into the nature of the genuine Mott state. Combining optical spectroscopy with pressure-dependent dc transport and theoretical calculations, we succeeded to construct a phase diagram valid for all Mott insulators on a quantitative scale. Our findings reveal the Pomeranchuk-like anomaly of the Mott transition and metallic fluctuations within the Mott gap, previously predicted but never observed.

Presenters

  • Andrej Pustogow

    University of Stuttgart

Authors

  • Andrej Pustogow

    University of Stuttgart

  • Mathias Bories

    University of Stuttgart

  • Anja Löhle

    University of Stuttgart

  • Roland Rösslhuber

    University of Stuttgart

  • Elena Zhukova

    Moscow Institute of Physics and Technology

  • Boris Gorshunov

    Moscow Institute of Physics and Technology

  • Silvia Tomic

    Institut za fiziku

  • John Schlueter

    Division of Materials Research, National Science Foundation, Materials Science Division, Argonne National Laboratory, Argonne

  • Ralph Hübner

    University of Stuttgart

  • Takaaki Hiramatsu

    Meijo University

  • Yukihiro Yoshida

    Meijo University

  • Gunzi Saito

    Meijo University, Meijo Univ

  • Reizo Kato

    RIKEN, Condensed Molecular Materials Labolatory, RIKEN

  • Tsung-Han Lee

    Florida State University

  • Vladimir Dobrosavljevic

    Florida State University

  • Simone Fratini

    Institut Neel, Universite Grenoble Alpes

  • Martin Dressel

    University of Stuttgart