Gating and superlattice effects in monolayer WSe2 devices in micro-ARPES

ORAL

Abstract

We investigate the effects of electrostatic doping and moiré superlattice potentials on monolayer WSe2 using micro-angle-resolved photoemission spectroscopy (micro-ARPES). By employing a local back gate of thin graphite under a hexagonal boron nitride dielectric support, we electrostatically populate the WSe2 conduction band during the photoemission measurements. We find the conduction band edge to be at the zone corner, or K point, confirming the direct gap nature of this material and yielding a measurement of the single-particle gap. As the electron doping is increased to a maximum of ~1.4E13 cm-2 the valence band shifts upwards towards the conduction band, corresponding to substantial band gap renormalization. At the highest doping levels, the conduction band minimum at the lower symmetry Q point is also populated, showing that it is within ∼30 meV of the minimum at K. In some devices we also observe folded copies of the hBN and WSe2 bands with intensities often comparable to the original bands, yielding information about moire superlattice effects.

Presenters

  • Paul Nguyen

    University of Washington

Authors

  • Paul Nguyen

    University of Washington

  • Natalie Teutsch

    Physics, University of Warwick

  • Abigail J Graham

    Physics, University of Warwick

  • Minhao He

    University of Washington

  • Viktor Kandyba

    Elettra-Sincrotrone Trieste, Elettra - Sincrotrone Trieste S.C.p.A

  • Alexei Victorovich Barinov

    Elettra-Sincrotrone Trieste, Elettra - Sincrotrone Trieste S.C.p.A

  • Neil R Wilson

    Physics, University of Warwick

  • Xiaodong Xu

    Physics, University of Washington, Seattle, University of Washington

  • David Henry Cobden

    University of Washington